疏水型氨基杂化SiO2气凝胶制备及CO2吸附性能任务书
2020-07-02 10:07
1. 毕业设计(论文)的内容和要求
co2是导致全球变暖和气候问题的主要温室气体之一。
大气中co2的浓度在过去几十年正在加速增长,导致全球范围内的气候问题和自然灾害频现。
co2捕集可以减少碳排放,缓解全球变暖的进程及其危害。
2. 参考文献
[1] G.T. Rochelle. Amine scrubbing for CO2 capture [J]. Science, 2009, 325(5948): 1652-1654. [2] K.E. Zanganeh, A. Shafeen, C. Salvador. CO2 Capture and development of an advanced pilot-scale cryogenic separation and compression unit [J]. Energy Procedia, 2009, 1(1): 247-252. [3] T.H. Bae, J.S. Lee, W. Qiu, et al. A high-performance gas-separation membrane containing submicrometer-sized metal-organic framework crystals [J]. Angewandte Chemie International Edition, 2010, 49(51): 9863-9866. [4] M.C. Stern, F. Simeon, H. Herzog, et al. Post-combustion carbon dioxide capture using electrochemically mediated amine regeneration [J]. Energy Environmental Science, 2013, 6(8): 2505-2517. [5] G. Qi, Y. Wang, L. Estevez, et al. High efficiency nanocomposite sorbents for CO2 capture based on amine-functionalized mesoporous capsules [J]. Energy Environmental Science, 2011, 4(2): 444-452. [6] Y. Kong, X. Shen, S. Cui, et al. Use of monolithic silicon carbide aerogel as a reusable support for development of regenerable CO2 adsorbent [J]. RSC Advances, 2014, 4(109): 64193-64199. [7] O. Shekhah, Y. Belmabkhout, Z.J. Chen, et al. Made-to-order metal-organic frameworks for trace carbon dioxide removal and air capture [J]. Nature Communications, 2014, 5: 4228. [8] Y. Kong, G. Jiang, M. Fan, et al. A new aerogel based CO2 adsorbent developed using a simple sol-gel method along with supercritical drying [J]. Chemical Communications, 2014, 50(81): 12158-12161. [9] N. Hedin, L. Andersson, L. Bergstr鰉, et al. Adsorbents for the post-combustion capture of CO2 using rapid temperature swing or vacuum swing adsorption [J]. Applied Energy, 2013, 104: 418-433. [10] F. Raganati, P. Ammendola, R. Chirone. CO2 adsorption on fine activated carbon in a sound assisted fluidized bed: Effect of sound intensity and frequency, CO2 partial pressure and fluidization velocity [J]. Applied Energy, 2014, 113: 1269-1282. [11] X.Q. Fan, L.X. Zhang, G.B. Zhang, et al. Chitosan derived nitrogen-doped microporous carbons for high performance CO2 capture [J]. Carbon, 2013, 61: 423-430. [12] S. Choi, J.H. Drese, C.W. Jones. Adsorbent materials for carbon dioxide capture from large anthropogenic point sources [J]. ChemSusChem, 2009, 2(9): 796-854. [13] A. Sayari, Y. Belmabkhout. Stabilization of amine-containing CO2 adsorbents: dramatic effect of water vapor [J]. Journal of the American Chemical Society, 2010, 132(18): 6312-6314. [14] M. Radosz, X.D. Hu, K. Krutkramelis, et al. Flue-gas carbon capture on carbonaceous sorbents: Toward a low-cost multifunctional carbon filter for "green" energy producers [J]. Industrial Engineering Chemistry Research, 2008, 47(10): 3783-3794. [15] N.A. Brunelli, S.A. Didas, K. Venkatasubbaiah, et al. Tuning cooperativity by controlling the linker length of silica-supported amines in catalysis and CO2 capture [J]. Journal of the American Chemical Society, 2012, 134(34): 13950-13953. [16] F. Rezaei, R.P. Lively, Y. Labreche, et al. Aminosilane-grafted polymer/silica hollow fiber adsorbents for CO2 capture from flue gas [J]. Acs Applied Materials Interfaces, 2013, 5(9): 3921-3931. [17] S. Cui, W. Cheng, X. Shen, et al. Mesoporous amine-modified SiO2 aerogel: a potential CO2 sorbent [J]. Energy Environmental Science, 2011, 4(6): 2070-2074. [18] K. W鰎meyer, I. Smirnova. Adsorption of CO2, moisture and ethanol at low partial pressure using aminofunctionalised silica aerogels [J]. Chemical Engineering Journal, 2013, 225: 350-357. [19] R. Begag, H. Krutka, W. Dong, et al. Superhydrophobic amine functionalized aerogels as sorbents for CO2 capture [J]. Greenhouse Gases: Science and Technology, 2013, 3(1): 30-39. [20] N.N. Linneen, R. Pfeffer, Y. Lin. Amine distribution and carbon dioxide sorption performance of amine coated silica aerogel sorbents: effect of synthesis methods [J]. Industrial Engineering Chemistry Research, 2013, 52(41): 14671-14679. [21] N. Linneen, R. Pfeffer, Y. Lin. CO2 capture using particulate silica aerogel immobilized with tetraethylenepentamine [J]. Microporous and Mesoporous Materials, 2013, 176: 123-131. [22] Z. Wang, Z. Dai, J. Wu, et al. Vacuum-dried robust bridged silsesquioxane aerogels [J]. Advanced Materials, 2013, 25(32): 4494-4497.
3. 毕业设计(论文)进程安排
2017.12.11~2017.12.26 确定选题、下达任务书 2016.12.26~2017.1.13 完善课题研究方案、外文翻译、文献综述和开题报告等工作 2017.2.26~2017.6.14 开展实验研究、结果分析 完成中期检查工作 撰写、修改、完善毕业论文 答辩
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